李东亚,博士,特别教授,硕士生导师,湖北省楚天学者计划“楚天学子”,国家注册环保工程师。
从事水体污染控制理论与修复技术的相关研究工作,主要集中于工业废水深度处理及资源化技术的研究及推广应用。2019年获湖北省楚天学者计划资助,承担中央支持地方科技发展专项、湖北自然科学基金等项目10余项,累计经费800余万。相关成果已发表论文70余篇,其中近五年来以第一作者/通讯作者在《Journal of Materials Chemistry A》《Chemical Engineering Journal》《Carbon》《ACS Applied Materials & Interfaces》等知名刊物上发表高水平论文48篇;申请国家发明专利13项,其中11项已授权。
基于已有研究成果,形成的“高浓有毒有机废水氧化深度处理技术”等具有自主知识产权的新技术、新装备,已在全国多个省(区)的10多家企业应用,为我国的生态环境保护做出了积极努力的工作。
主要研究兴趣包括:
1.难降解工业废水深度处理技术,特别关注“风险与效应协同控制”等水处理新理论、新工艺和新装备;
2.新型环境功能材料在水污染控制与资源回收中的应用,重点关注碳中和、CO2捕获封存、废水处理及回用、清洁水生产等新兴领域的理论和方法;
3.催化行为的界面调控与机理解析,努力探索界面上电场构造及其对电子行为作用的微观过程;
4.太阳能耦合化学催化系统中污染物迁移转化行为及效应的环境地球化学过程,提出并深入研究以载流子-激子-声子耦合、污染物质流为主线的“生态通量”与过程调控机制。
联系方式:dyli@wtu.edu.cn。
欢迎上进心强、有相关研究兴趣和志向、乐观积极、执行力强、沟通意识强,具有较强的学习意愿的本科、研究生同学加入和咨询。
主要教学成果和荣誉
先后指导国家级、省级老员工创新创业项目5项,指导员工获挑战杯国家二等奖、湖北省特等奖等奖励多项。
1.指导员工获得第十六届“挑战杯”全国老员工课外科技作品竞赛二等奖,2019年。
2.指导员工获得湖北省第十二届“挑战杯”老员工课外科技作品竞赛特等奖,2019年。
3.指导员工获得g-C3N4复合Fe2O3结构调控及其催化单过硫酸盐降解双酚A的研究,2021年,国家级老员工创新创业项目。
4.指导员工获得硼表面掺杂铜氧化物的调控构筑及其催化单过硫酸盐降解双酚A的研究,2021年,省级老员工创新创业项目。
5.指导员工获得CuO-FeOCl异质场催化单过硫酸盐降解双酚A的研究,2021年,省级老员工创新创业项目。
6.指导员工获得g-C3N4-Cu2O的形貌调控及其可见光催化甲基橙(MO)的机制,2018年,省级老员工创新创业项目。
7.指导员工获得可见光协同FeOCl催化活化过氧化氢的机理研究,2018年,省级老员工创新创业项目。
8.指导学士学位论文《微波-紫外光耦合催化活化过一硫酸盐处理印染废水的研究》获湖北省优秀学士学位论文,2017年。
9.获得“beat365官方登录入口成果转化标兵”荣誉称号,2020年。
10.获得beat365官方登录入口“优秀指导老师”称号,2021年。
代表性学术论文
近五年来,相关成果以第一作者/通讯作者在《Journal of Materials Chemistry A》《Chemical Engineering Journal》《ACS Applied Materials & Interfaces》《Carbon》等知名刊物上发表论文48篇。代表性学术论文如下:
1.Shiyu Zuo, Zeyu Guan, Fan Yang, Dongsheng Xia,Dongya Li*. Reactive Oxygen Species Regulation and Synergistic for Effective Water Purification through Fenton-like Catalysis on Single-Atom Cu-N Sites [J]. Journal of Materials Chemistry A, 2022. (IF=12.732,中科院1区)
2.Shiyu Zuo,Dongya Li*,Zeyu Guan, Fan Yang, Junqi Song, Haiming Xu, Dongsheng Xia, Huanxuan Li, Xiaohu Li. A Directional Built-in Electric Field Mediates the Electron Transfer Synergy Mechanism of Radicals/Nonradicals Pathway in FeOCl-CuO [J]. Chemical Engineering Journal, 2022, 430: 133004.
3.Shiyu Zuo,Dongya Li*, Zeyu Guan, Fan Yang, Dongsheng Xia, Mingzhi Huang. Utilization of sewage resources through efficient solar-water evaporation by single-atom Cu sites[J]. Carbon, 2022, 187: 207-215.
4.Qihui Wang, Zeyu Guan, Su Ding, Dongsheng Xia,Dongya Li*. Tuning the Surface Electronic State by the introduction of Mn on Fe2O3to boost the Activity of Peroxymonosulfate[J]. Separation and Purification Technology, 2022: 120625.
5.Shiyu Zuo,Dongya Li*, Zeyu Guan, Yi Zhu, Mengjie Pu, Dongsheng Xia. Rapid electron transfer boosts CuO-Mediated nonradical oxidation pathways for efficient removal of Bisphenol[J]. Journal of Cleaner Production, 2022: 130480.
6.Yichen Ding,Dongya Li*, Shiyu Zuo, Zeyu Guan, Su Ding. Boron-doping accelerated Cu (II)/Cu (I) cycle for enhancing peroxymonosulfate activation[J]. Separation and Purification Technology,2022, 282: 120086.
7.Shiyu Zuo,Dongya Li*,Zeyu Guan, Fan Yang, Haiming Xu, Dongsheng Xia, Jinquan Wan. Tailored d‑Band Facilitating in Fe Gradient Doping CuO Boosts Peroxymonosulfate Activation for High Efficiency Generation and Release of Singlet Oxygen [J]. ACS Applied Materials & Interfaces, 2021, 13(42): 49982-49992. (Cover article)
8.Hui Song, Zeyu Guan, Luyi Chen, Haiming Xu, Dongsheng Xia, Mingzhi Huang,Dongya Li*.Role of curvature in a carbon electronic structure under spatial confinement: conversion of nonradicals to radicals [J]. Carbon, 2021, 180: 22-30.
9.Meng Li, Dongsheng Xia, Haiming Xu, Zeyu Guan,Dongya Li*.Iron oxychloride composite sludge-derived biochar for efficient activation of peroxymonosulfate to degrade organic pollutants in wastewater[J]. Journal of Cleaner Production,2021, 329: 129656.
10.Shiyu Zuo, Zeyu Guan, Dongsheng Xia*, Fan Yang, Haiming Xu, Mingzhi Huang,Dongya Li*. Polarized heterogeneous CuO-CN for peroxymonosulfate nonradical activation: An enhancement mechanism of mediated electron transfer[J]. Chemical Engineering Journal, 2021: 127619.
11.Hui Song, Zhuang Liu, Zeyu Guan, Fan Yang, Dongsheng Xia,Dongya Li*. Efficient persulfate non-radical activation of electron-rich copper active sites induced by oxygen on graphitic carbon nitride[J]. Science of The Total Environment, 2021, 762: 143127.
12.Shiyu Zuo, Jie Zan,Dongya Li*,Zeyu Guan, Fan Yang, Haiming Xu, Mingzhi Huang, Dongsheng Xia. Efficient Peroxymonosulfate Nonradical Activity of Zn-Mn-Al2O3@g-C3N4via Synergism of Zn, Mn doping and g-C3N4composite [J]. Separation and Purification Technology, 2021: 118965.
13.Shiyu Zuo, Dongsheng Xia, Zeyu Guan, Fan Yang, Binyang Zhang, Haiming Xu, Mingzhi Huang, Xuetao Guo,Dongya Li*. The Polarized Electric Field on Fe2O3/g-C3N4for Efficient Peroxymonosulfate Activation: A Synergy of1O2, Electron transfer and Pollutant Oxidation[J]. Separation and Purification Technology, 2021: 118717.
14.Shiyu Zuo,Dongya Li*, Fan Yang, Haiming Xu, Mingzhi Huang, Zeyu Guan*, Dongsheng Xia. Copper Oxide/Graphitic Carbon Nitride Composite for Bisphenol A Degradation by Boosted Peroxymonosulfate Activation: Mechanism of Cu-O Covalency Governs [J]. Journal of Colloid and Interface Science, 2021.
15.Zeyu Guan, Shiyu Zuo, Fan Yang, Binyang Zhang, Haiming Xu, Dongsheng Xia*, Mingzhi Huang,Dongya Li*. The p and d hybridization interaction in Fe-N-C boosts peroxymonosulfate non-radical activation[J]. Separation and Purification Technology, 2021, 258: 118025.
16.Hui Song, Zeyu Guan, Dongsheng Xia*, Haiming Xu, Fan Yang,Dongya Li*, Xiaohu Li. Copper-oxygen synergistic electronic reconstruction on g-C3N4for efficient non-radical catalysis for peroxydisulfate and peroxymonosulfate[J]. Separation and Purification Technology, 2021, 257: 117957.
17.Shiyu Zuo, Dongsheng Xia, Zeyu Guan, Fan Yang, Shuang Cheng, Haiming Xu, Renzhuo Wan*,Dongya Li*, Min Liu. Dual-functional CuO/CN for highly efficient solar evaporation and water purification[J]. Separation and Purification Technology, 2021, 254: 117611.
18.Yi Zhu,Dongya Li*, Shiyu Zuo, Zeyu Guan, Su Ding, Dongsheng Xia, Xiaohu Li.Cu2O/CuO induced non-radical/radical pathway toward highly efficient peroxymonosulfate activation[J]. Journal of Environmental Chemical Engineering,2021.11.
19.Shiyu Zuo,Dongya Li*, Haiming Xu, Dongsheng Xia*. An integrated microwave-ultraviolet catalysis process of four peroxides for wastewater treatment: Free radical generation rate and mechanism[J]. Chemical Engineering Journal, 2020, 380: 122434.
20.Jie Zan, Hui Song, Shiyu Zuo, Xiangrui Chen, Dongsheng Xia*,Dongya Li*. MIL-53 (Fe)-derived Fe2O3with oxygen vacancy as Fenton-like photocatalysts for the elimination of toxic organics in wastewater[J]. Journal of Cleaner Production, 2020, 246: 118971.
21.Dongya Li*, Jie Zan, Liping Wu, Shiyu Zuo, Haiming Xu*, and Dongsheng Xia*. Heterojunction tuning and catalytic efficiency ofg-C3N4-Cu2Owith glutamate[J]. Industrial & Engineering Chemistry Research, 2019, 58(10): 4000-4009.
22.Dongya Li,Shiyu Zuo, Haiming Xu*, Jie Zan, Lei Sun, Donghui Han, Wei Liao, Binyang Zhang, Dongsheng Xia*. Synthesis of a g-C3N4-Cu2O heterojunction with enhanced visible light photocatalytic activity by PEG [J]. Journal of colloid and interface science, 2018, 531: 28-36.
专利成果
以第一发明人申请国家发明专利13项,其中已授权11项。
1.李东亚;夏东升;徐海明;袁向娟;曹刚;孙磊;陈梦蝶;王琦.[中国发明],专利号:CN201611225263.8.
2.李东亚;夏东升;徐海明;袁向娟;曹刚;孙磊;陈梦蝶.[中国发明],专利号:CN201611224567.2.
3.李东亚;夏东升;徐海明;袁向娟;孙磊;曹刚;陈梦蝶;王琦.[中国发明],专利号:CN201611224587.X
4.李东亚;夏东升;徐海明;袁向娟;孙磊;曹刚;陈梦蝶.[中国发明],专利号:CN201611224577.6.
5.李东亚;夏东升;徐海明;廖伟;左诗语;曹刚;袁向娟;孙磊.[中国发明],专利号:CN201710483431.1.
6.李东亚;夏东升;徐海明;廖伟;左诗语;曹刚;袁向娟;孙磊;武利平.[中国发明],专利号:CN201710479044.0
7.李东亚;夏东升;徐海明;左诗语;廖伟;曹刚;袁向娟;孙磊;武利平[中国发明],专利号:CN201710479020.5.
8.李东亚;夏东升;徐海明;曹刚;袁向娟;孙磊;廖伟;左诗语;武利平[中国发明],专利号:CN201710479053.X.
9.李东亚;夏东升;徐海明;左诗语;廖伟;曹刚;袁向娟;孙磊[中国发明],专利号:CN201710479009.9.
10.李东亚;夏东升;左诗语;徐海明;孙磊[中国发明],专利号:CN201910502983.1.
11.李东亚;夏东升;左诗语;徐海明;孙磊[中国发明],专利号:CN201910502978.0.
主要的科研项目
1.湖北省科技厅重大专项:基于电荷自循环的有毒有机物绿色催化脱毒及生态保障技术应用研究(1920001000160),2020/12—2022/12。
2.湖北省自然科学基金:Cu/Fe-g-C3N4催化过硫酸盐的活性位点调控及微观机制研究,2018/03—2020/03。
3.湖北老磨坊豆制品有限公司水处理系统改造,2020/07—2020/09。
4.印染废水深度氧化处理技术及设备研发,2021/04—2022/01。
5.含硫难降解印染废水整体处理技术及设备集成示范项目,2021/01—2021/05。
6.难降解工业废水高级氧化一体化深度处理及资源化技术研发,2020/12—2021/05。
7.新型造纸废水深度氧化处理技术应用,2020/12—2021/05。
8.难降解工业废水高级氧化深度处理技术,2020/12—2021/01。
9.水性砂壁浆涂料生产废水达标回用项目,2020/11—2021/05。
10.造纸浆塔设备制造技术服务,2020/07—2021/07。
11.污水站技术及维修服务项目,2020/06—2021/09。
12.工业废水总体设计及一体化沉降设备制造、运行指导,2020/05—2020/06。
13.造纸废水深度处理厌氧处理技术开发及示范,2021/12—2022/12。
社会任职
担任Environ. Sci. Technol、J Mater Chem A、Chem. Eng. J、J. Hazard. Mater、Water. Res等十余种SCI期刊审稿人。